A2 Refereed review article in a scientific journal

Plant-Based Structures as an Opportunity to Engineer Optical Functions in Next-Generation Light Management




AuthorsKaschuk Joice Jaquelin, Al Haj Yazan, Rojas Orlando J., Miettunen Kati, Abitbol Tiffany, Vapaavuori Jaana

PublisherWiley-VCH

Publication year2022

JournalAdvanced Materials

Journal name in sourceADVANCED MATERIALS

Journal acronymADV MATER

Article numberARTN 2104473

Number of pages37

ISSN0935-9648

eISSN1521-4095

DOIhttps://doi.org/10.1002/adma.202104473

Self-archived copy’s web addresshttps://research.utu.fi/converis/portal/detail/Publication/68686344


Abstract
This review addresses the reconstruction of structural plant components (cellulose, lignin, and hemicelluloses) into materials displaying advanced optical properties. The strategies to isolate the main building blocks are discussed, and the effects of fibrillation, fibril alignment, densification, self-assembly, surface-patterning, and compositing are presented considering their role in engineering optical performance. Then, key elements that enable lignocellulosic to be translated into materials that present optical functionality, such as transparency, haze, reflectance, UV-blocking, luminescence, and structural colors, are described. Mapping the optical landscape that is accessible from lignocellulosics is shown as an essential step toward their utilization in smart devices. Advanced materials built from sustainable resources, including those obtained from industrial or agricultural side streams, demonstrate enormous promise in optoelectronics due to their potentially lower cost, while meeting or even exceeding current demands in performance. The requirements are summarized for the production and application of plant-based optically functional materials in different smart material applications and the review is concluded with a perspective about this active field of knowledge.

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