A1 Vertaisarvioitu alkuperäisartikkeli tieteellisessä lehdessä

Spatial Diffusion of Hydrogen Atoms in Normal and Para-Hydrogen Molecular Films at Temperature 0.7 K




TekijätSheludiakov S., Wetzel C. K., Lee D. M., Khmelenko V. V., Järvinen J., Ahokas J., Vasiliev S.

KustantajaSpringer Nature

Julkaisuvuosi2024

JournalJournal of Low Temperature Physics

Tietokannassa oleva lehden nimiJOURNAL OF LOW TEMPERATURE PHYSICS

Lehden akronyymiJ LOW TEMP PHYS

Vuosikerta215

Numero5-6

Aloitussivu336

Lopetussivu356

Sivujen määrä21

ISSN0022-2291

eISSN1573-7357

DOIhttps://doi.org/10.1007/s10909-024-03053-w

Verkko-osoitehttps://link.springer.com/article/10.1007/s10909-024-03053-w

Rinnakkaistallenteen osoitehttps://research.utu.fi/converis/portal/detail/Publication/387220279


Tiivistelmä

We report on electron spin resonance studies of H atoms stabilized in solid H2 flms at temperature 0.7 K and in a magnetic feld of 4.6 T. The H atoms were produced by bombarding H2 flms with 100 eV electrons from a radiofrequency discharge run in the sample cell. We observed a one order of magnitude faster H atom accumulation in the flms made of para-H2 gas with a small ortho-H2 concentration (0.2% ortho-H2) as compared with those made from normal H2 gas content (75% ortho-H2). We also studied the infuence of ortho-H2 molecules on spatial difusion of H atoms in solid H2 flms. The spatial difusion of H atoms in both normal and para-H2 flms is faster than the difusion obtained from the measurement of H atom recombination. The rate of spatial difusion of H atoms in para-H2 flms was slower in comparison with that in the normal H2 flms. We discuss possible explanations of these observations. 


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