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Purely Spatial Quantum Diffusion of H Atoms in Solid H-2 at Temperatures below 1 K




TekijätSheludiakov Sergei, Lee D. M., Khmelenko Vladimir V., Järvinen Jarno, Ahokas Janne, Vasiliev Sergey

KustantajaAMER PHYSICAL SOC

Julkaisuvuosi2021

JournalPhysical Review Letters

Tietokannassa oleva lehden nimiPHYSICAL REVIEW LETTERS

Lehden akronyymiPHYS REV LETT

Artikkelin numeroARTN 195301

Vuosikerta126

Numero19

Sivujen määrä5

ISSN0031-9007

eISSN1079-7114

DOIhttps://doi.org/10.1103/PhysRevLett.126.195301

Rinnakkaistallenteen osoitehttps://research.utu.fi/converis/portal/detail/Publication/59546959


Tiivistelmä
We report on a direct measurement of the quantum diffusion of H atoms in solid molecular hydrogen films at T = 0.7 K. We obtained a rate of pure spatial diffusion of H atoms in the H-2 films, D-d = 5(2) x 10(-17) cm(2) s(-1), which was 2 orders of magnitude faster than that obtained from H atom recombination, the quantity used in all previous work to characterize the mobility of H atoms in solid H-2. We also observed that the H-atom diffusion was significantly enhanced by injection of phonons. Our results provide the first measurement of the pure spatial diffusion rate for H atoms in solid H-2, the only solid state system beside He-3 - He-4 mixtures, where atomic diffusion does not vanish even at temperatures below 1 K.

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