A1 Refereed original research article in a scientific journal

Two mirror X-ray pulse split and delay instrument for femtosecond time resolved investigations at the LCLS free electron laser facility




AuthorsBerrah N, Fang L, Murphy BF, Kukk E, Osipov TY, Coffee R, Ferguson KR, Xiong H, Castagna JC, Petrovic VS, Montero SC, Bozek JD

PublisherOPTICAL SOC AMER

Publication year2016

JournalOptics Express

Journal name in sourceOPTICS EXPRESS

Journal acronymOPT EXPRESS

Volume24

Issue11

First page 1768

Last page1781

Number of pages14

ISSN1094-4087

eISSN1094-4087

DOIhttps://doi.org/10.1364/OE.24.011768


Abstract
We built a two-mirror based X-ray split and delay (XRSD) device for soft X-rays at the Linac Coherent Light Source free electron laser facility. The instrument is based on an edge-polished mirror design covering an energy range of 250 eV-1800 eV and producing a delay between the two split pulses variable up to 400 femtoseconds with a sub-100 attosecond resolution. We present experimental and simulation results regarding molecular dissociation dynamics in CH3I and CO probed by the XRSD device. We observed ion kinetic energy and branching ratio dependence on the delay times which were reliably produced by the XRSD instrument. (C)2016 Optical Society of America

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